The Fermi–Löwdin self-interaction correction for ionization energies of organic molecules

Abstract

(Semi)-local density functional approximations (DFAs) suffer from self-interaction error (SIE). When the first ionization energy (IE) is computed as the negative of the highest-occupied orbital (HO) eigenvalue, DFAs notoriously underestimate them compared to quasi-particle calculations. The inaccuracy for the HO is attributed to SIE inherent in DFAs. We assessed the IE based on Perdew–Zunger self-interaction correction on 14 small to moderate-sized organic molecules relevant in organic electronics and polymer donor materials. Although self-interaction corrected DFAs were found to significantly improve the IE relative to the uncorrected DFAs, they overestimate. However, when the self-interaction correction is interiorly scaled using a function of the iso-orbital indicator zσ, only the regions where SIE is significant get a correction. We discuss these approaches and show how these methods significantly improve the description of the HO eigenvalue for the organic molecules.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 10, 2020
Source ID
10.1063/5.0024776

Entities

People

  • Adrienn Ruzsinszky
  • Biswajit Santra
  • Koblar Alan Jackson
  • Niraj K Nepal
  • Puskar Bhattarai
  • Santosh Adhikari
  • Shiqi Ruan

Organizations

  • Central Michigan University
  • National Science Foundation
  • Temple University
  • United States Department of Energy

Tags

Readers

  • Marine Ecological Systems Migration
  • Quantum Chemistry
  • Regression Analysis.

Technology Areas

  • Microelectronics
  • Space