Near-field imaging of plasmonic nanopatch antennas with integrated semiconductor quantum dots
Abstract
Plasmonic nanopatch antennas that incorporate dielectric gaps hundreds of picometers to several nanometers thick have drawn increasing attention over the past decade because they confine electromagnetic fields to grossly sub-diffraction-limited volumes. Substantial control over the optical properties of excitons and color centers confined within these plasmonic cavities has already been demonstrated with far-field optical spectroscopies, but near-field optical spectroscopies are essential for an improved understanding of the plasmon–emitter interaction at the nanoscale. Here, we characterize the intensity and phase-resolved plasmonic response of isolated nanopatch antennas by cathodoluminescence microscopy. Furthermore, we explore the distinction between optical and electron beam spectroscopies of coupled plasmon–exciton heterostructures to identify constraints and opportunities for future nanoscale characterization and control of hybrid nanophotonic structures. While we observe substantial Purcell enhancement in time-resolved photoluminescence spectroscopies, negligible Purcell enhancement is observed in cathodoluminescence spectroscopies of hybrid nanophotonic structures. The substantial differences in measured Purcell enhancement for electron beam and laser excitation can be understood as a result of the different selection rules for these complementary experiments. These results provide a fundamentally new understanding of near-field plasmon–exciton interactions in nanopatch antennas, which is essential for myriad emerging quantum photonic devices.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Oct 01, 2021
- Source ID
- 10.1063/5.0065524
Entities
People
- Andrew Butler
- Ben Lawrie
- Brian E. Lerner
- Christos Argyropoulos
- Jiyang Chen
- Thang B. Hoang
- Vasudevan Iyer
- Yoong Sheng Phang
Organizations
- Duke University
- National Science Foundation
- Oak Ridge National Laboratory
- Office of Basic Energy Sciences
- Office of Naval Research
- Quantum Science Center
- University of Georgia
- University of Memphis
- University of Nebraska–Lincoln