Spiropyran-functionalized photochromic nylon webbings for long-term ultraviolet light sensing

Abstract

Webbing structures are extensively employed in engineering systems as load-bearing components. In a field setting, webbings are frequently subject to extended ultraviolet (UV) light irradiation, which can affect their integrity and reduce their mechanical strength. Despite technological advancements in structural health monitoring, long-term UV sensing techniques for webbings remain under-developed. To fill this gap, we propose a photochromic nylon webbing that demonstrates color variation in response to extended UV exposure. The webbing offers a rich, yet controlled, color variation over multiple time scales that is conducive to UV sensing. A mathematical model grounded in photochemistry is developed to interpret experimental observations, unveiling the photochromic phenomenon as a multi-step, multi-timescale photochemical process involving several chemical species. The model captures the evolution of the coexisting species through a system of nonlinear, coupled ordinary differential equations, offering the basis for the inference of the webbing’s color. The proposed photochromic webbing and the photochemistry-based mathematical model could inform future designs of UV-sensitive structures that maintain sensitivity under weeks of continuous sunlight UV exposure.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 08, 2022
Source ID
10.1063/5.0093641

Entities

People

  • Maurizio Porfiri
  • Osgar John Ohanian Iii
  • Peng Zhang

Organizations

  • Luna Innovations Incorporated
  • New York University
  • United States Navy

Tags

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Distributed Systems and Data Platform Development
  • Explosive Engineering.

Technology Areas

  • AI & ML
  • AI & ML - Autonomous Systems
  • AI & ML - Bayesian Inference