Shock ignition and deflagration growth in plastic-bonded TATB (1, 3, 5-trinitro-2, 4, 6-triaminobenzene) microstructures

Abstract

TATB (1,3,5-triamino-2,4,6-trinitrobenzene) plastic-bonded explosives (PBX) were shocked with laser-launched flyer plates. The spectral radiance of the emitted light from a small portion of the microstructure (a “microenvironment”) containing a small number of TATB particles with an estimated mass of 150 ng was measured every 0.8 ns from 1 ns to 200 μs and was analyzed to give radiance and time-dependent graybody temperatures. By fabricating an array with 186 PBX charges, we could obtain ≥15 shots at each of 12 velocities between 1.8 and 4.7 km/s. We found that every microenvironment generated a unique radiance fingerprint. Some of these microenvironments were much more reactive than average. The radiance has two peaks around 20 ns and 5 μs, associated with shock ignition and deflagration growth. In our interpretation, the shock creates an ensemble of hot spots of various sizes and temperatures. Of those hot spots that ignite, only a small portion, at about 2200 K, was large enough and hot enough to survive long enough (>100 ns) to ignite individual TATB particles, leading to deflagration. Integrating various time intervals of the radiance can quantify the strength of the shock–PBX interaction, and the decay and growth of the hot spot ensemble and the deflagration.

Document Details

Document Type
Pub Defense Publication
Publication Date
Aug 08, 2022
Source ID
10.1063/5.0101248

Entities

People

  • Dana D. Dlott
  • Lawrence Salvati
  • Meysam Akhtar
  • Siva Kumar Valluri

Organizations

  • Air Force Office of Scientific Research
  • Lawrence Livermore National Laboratory
  • University of Illinois Urbana–Champaign

Tags

Fields of Study

  • Physics

Readers

  • Aerosol Science/Aerosol Physics
  • Combustion Dynamics and Shock Wave Physics.
  • Spectroscopy.

Technology Areas

  • Directed Energy