Fabrication of interdigitated electrodes of graphene oxide/silica by femtosecond laser-induced forward transfer for sensing applications

Abstract

Graphene-based materials, such as graphene oxide (GO), have been receiving much attention due to their graphene-like properties and compatibility with other materials. At the same time, novel printing methods have been developed for fabricating high-resolution patterns, such as Laser-Induced Forward Transfer (LIFT), which allows microscale transferring of a variety of materials to distinct substrates, enabling the design of micro- and nanodevices for biomedical and opto-electronic application. In this work, we propose the use of LIFT with fs-laser pulses for creating high-resolution interdigitated electrodes of tetraethyl orthosilicate functionalized with GO. The fs-LIFT approach successfully allowed micro-patterning of lines with widths on the order of 2 μm, with threshold energy of 70 nJ, and the reduction of graphene oxide to fabricate silica/GO films in an efficient, controlled, and localized way, without material degradation. As a proof of principle, interdigitated electrodes fabricated by fs-LIFT were successfully used as the sensing units of an impedimetric electronic tongue for taste recognition and heavy metals ions detection (Al3+, Hg2+, Co2+, and Cu2+) at different concentrations of 100 nmol l−1, 10 μmol l−1, and 1 mmol l−1.

Document Details

Document Type
Pub Defense Publication
Publication Date
Feb 06, 2023
Source ID
10.1063/5.0137926

Entities

People

  • Cleber R Mendonca
  • Daniel S. Correa
  • Francineide Lopes de Araújo
  • Kelly T. Paula
  • Marcelo B Andrade
  • Murilo H.M. Facure
  • Sabrina Nicoleti Carvalho dos Santos

Organizations

  • Air Force Office of Scientific Research
  • Coordenação de Aperfeicoamento de Pessoal de Nível Superior
  • Embrapa
  • National Council for Scientific and Technological Development
  • São Paulo Research Foundation
  • United States Army Research Laboratory
  • University of São Paulo

Tags

Fields of Study

  • Materials science

Readers

  • Nanocomposite Materials Science
  • Nanofabrication and Microfabrication.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Biotechnology
  • Biotechnology - Bioremediation
  • Directed Energy
  • Microelectronics
  • Microelectronics - Graphene
  • Microelectronics - Microelectromechanical Systems