Ferroelectric domain wall dynamics characterized with X-ray photon correlation spectroscopy

Abstract

The dynamics in many complex systems is essentially heterogeneous and involves a series of discrete events—in particular, local structural changes. The nature and scale of these changes may vary greatly, ranging from rearrangements of atomic positions during phase transitions to displacements of tectonic plates during earthquakes. In this work, we introduce X-ray photon correlation spectroscopy (XPCS) as a powerful tool for investigating heterogeneous dynamics of interfaces. We observe the motion of ferroelectric domain walls by means of XPCS and obtain the information about nanoscale changes, which is inaccessible for other techniques. Further experiments can provide important insights into the mechanisms of unusual properties of materials such as anomalously large piezoelectric response in relaxor-based ferroelectrics and magnetoelectric coupling in multiferroics.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jul 03, 2018
Source ID
10.1073/pnas.1720991115

Entities

People

  • Alexei A Bokov
  • Alexey V. Zozulya
  • Arman Davtyan
  • Christian Gutt
  • Mario Reiser
  • Michael Sprung
  • Semen Gorfman
  • Ullrich Pietsch
  • Yujuan Xie
  • Zuo-Guang Ye

Organizations

  • DESY
  • European XFEL
  • Federal Ministry of Research, Technology and Space
  • Natural Sciences and Engineering Research Council
  • Office of Naval Research
  • Simon Fraser University
  • Tel Aviv University
  • University of Siegen

Tags

Fields of Study

  • Physics

Readers

  • Computational Fluid Dynamics (CFD)
  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics