Synergistic boost of output power density and efficiency in In-Li–codoped SnTe

Abstract

In the search for high-performance thermoelectric materials, in addition to conversion efficiency, output power density is also an important consideration for practical applications in generating electrical energy from solar or waste heat. We designed and fabricated an SnTe-based material that exhibits both high conversion efficiency and high output power density by indium and lithium codoping. Indium doping realizes the resonant state in the compound, while lithium doping further increases its carrier concentration by acting as an acceptor as well as dramatically reducing its lattice thermal conductivity by forming disperse precipitates. This work provides an example for finding high-performance thermoelectric materials that are suitable for practical application and provides guidance for future research.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 14, 2019
Source ID
10.1073/pnas.1911085116

Entities

People

  • Bo Cui
  • Bo Yu
  • Ching-Wu Chu
  • Fengkai Guo
  • Haijun Wu
  • Honghao Yao
  • Jianbo Zhu
  • Jiehe Sui
  • Qian Zhang
  • Stephen J. Pennycook
  • Wei Cai
  • Yang Zhang

Organizations

  • Air Force Office of Scientific Research
  • Harbin Institute of Technology
  • National Natural Science Foundation of China
  • University of Houston

Tags

Fields of Study

  • Materials science

Readers

  • Electrical Engineering
  • Materials Science and Engineering.
  • Systems Analysis and Design