Generalized scaling of spin qubit coherence in over 12,000 host materials
Abstract
Atomic defects in solid-state materials are promising candidates as quantum bits, or qubits. New materials are actively being investigated as hosts for new defect qubits; however, there are no unifying guidelines that can quantitatively predict qubit performance in a new material. One of the most critical property of qubits is their quantum coherence. While cluster correlation expansion (CCE) techniques are useful to simulate the coherence of electron spins in defects, they are computationally expensive to investigate broad classes of stable materials. Using CCE simulations, we reveal a general scaling relation between the electron spin coherence time and the properties of qubit host materials that enables rapid and quantitative exploration of new materials hosting spin defects.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Apr 06, 2022
- Source ID
- 10.1073/pnas.2121808119
Entities
People
- Christopher P Anderson
- David Awschalom
- F Joseph Heremans
- Gary Wolfowicz
- Giulia Galli
- Hideo Ōno
- Hosung Seo
- Mykyta Onizhuk
- Sean E. Sullivan
- Shun Kanai
Organizations
- Air Force Office of Scientific Research
- Ajou University
- Argonne National Laboratory
- Office of Basic Energy Sciences
- Office of Science
- Tohoku University
- University of Chicago