Epitaxial SrTiO 3 films with dielectric constants exceeding 25,000

Abstract

Semiconductor interfaces are among the most important in use in modern technology. The properties they exhibit can either enable or disable the characteristics of the materials they connect for functional performance. While much is known about important junctions involving conventional semiconductors such as Si and GaAs, there are several unsolved mysteries surrounding interfaces between oxide semiconductors. Here we resolve a long-standing issue concerning the measurement of anomalously low dielectric constants in SrTiO 3 films with record high electron mobilities. We show that the junction between doped and undoped SrTiO 3 required to make dielectric constant measurements masks the dielectric properties of the undoped film. Through modeling, we extract the latter and show that it is much higher than previously measured.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jun 02, 2022
Source ID
10.1073/pnas.2202189119

Entities

People

  • Bharat Jalan
  • Dooyong Lee
  • Jin Yue
  • Judith Gabel
  • Richard D. James
  • Scott A. Chambers
  • Tien-lin Lee
  • Zhifei Yang

Organizations

  • Air Force Office of Scientific Research
  • Diamond Light Source
  • National Science Foundation Directorate for Mathematical & Physical Sciences
  • Pacific Northwest National Laboratory
  • United States Department of Energy
  • University of Minnesota

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Theoretical Analysis.
  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene