Electronic structure in a transition metal dipnictide TaAs2

Abstract

The family of transition-metal dipnictides has been of theoretical and experimental interest because this family hosts topological states and extremely large magnetoresistance (MR). Recently, T a A s 2 , a member of this family, has been predicted to support a topological crystalline insulating state. Here, by using high-resolution angle-resolved photoemission spectroscopy (ARPES), we reveal both closed and open pockets in the metallic Fermi surface (FS) and linearly dispersive bands on the ( 2 ‾ 01 ) surface, along with the presence of extreme MR observed from magneto-transport measurements. A comparison of the ARPES results with first-principles computations shows that the linearly dispersive bands on the measured surface of T a A s 2 are trivial bulk bands. The absence of symmetry-protected surface state on the ( 2 ‾ 01 ) surface indicates its topologically dark nature. The presence of open FS features suggests that the open-orbit fermiology could contribute to the extremely large MR of T a A s 2 .

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 14, 2023
Source ID
10.1088/1361-648x/ad04fc

Entities

People

  • Anup Pradhan Sakhya
  • Arun Bansil
  • Bahadur Singh
  • BaoKai Wang
  • Cheng-yi Huang
  • Dariusz Kaczorowski
  • J F Mitchell
  • Jesse E. Thompson
  • Jonathan D Denlinger
  • M. Mofazzel Hosen
  • Madhab Neupane
  • Masahiro Ishigami
  • Mojammel A. Khan
  • Sabin Regmi

Organizations

  • Air Force Office of Scientific Research
  • Department of Atomic Energy
  • Division of Materials Research
  • Office of Basic Energy Sciences
  • Office of Science

Tags

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Space