Enhanced Dielectric and Ferroelectric Properties of Pb(Mg1/3Nb2/3)0.65Ti0.35O3 Ceramics by ZnO Modification

Abstract

Phase formation, microstructures, dielectric, and ferroelectric properties of ZnO‐modified Pb(Mg1/3Nb2/3)0.65Ti0.35O3 (PMNT/xZnO, where x = 0, 0.4, 2.0, 4.0, and 11.0 mol%) ceramics were studied. A coexistence of rhombohedral and tetragonal ferroelectric phases was observed at room temperature in all samples. The ceramics with the relative densities of 93%–95% were prepared. The modification by ZnO led to an increase in grain sizes of PMNT ceramics. The maximum dielectric constant of the pure PMNT ceramic was increased with x = 0.4–4.0 mol% ZnO doping, with the highest value being observed in the 2.0 mol% sample. Both the temperature at which the transition between rhombohedral and tetragonal ferroelectric phases took place (TR‐T) and the Curie temperature of the ceramics tended to increase with increasing x. The ferroelectric properties were enhanced with increased remanent polarization and P(E) loop squareness in the compositions with x = 0.4–4.0 mol%. However, the ferroelectric properties were attenuated with x = 11.0 mol%.

Document Details

Document Type
Pub Defense Publication
Publication Date
Dec 10, 2014
Source ID
10.1111/jace.13372

Entities

People

  • Anucha Watcharapasorn
  • Methee Promsawat
  • Sukanda Jiansirisomboon
  • Zuo‐guang Ye

Organizations

  • Chiang Mai University
  • Moscow Aviation Institute
  • Natural Sciences and Engineering Research Council
  • Office of Naval Research
  • Simon Fraser University
  • Thailand Research Fund

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Mathematics or Statistics