Applications of analytical electron microscopy to guide the design of boron carbide

Abstract

Compositional analysis of boron carbide on nanometer length scales to examine or interpret atomic mechanisms, for example, solid‐state amorphization or grain‐boundary segregation, is challenging. This work reviews advancements in high‐resolution microanalysis to characterize multiple generations of boron carbide. First, ζ‐factor microanalysis will be introduced as a powerful (scanning) transmission electron microscopy ((S)TEM) analytical framework to accurately characterize boron carbide. Three case studies involving the application of ζ‐factor microanalysis will then be presented: (1) accurate stoichiometry determination of B‐doped boron carbide using ζ‐factor microanalysis and electron energy loss spectroscopy, (2) normalized quantification of silicon grain‐boundary segregation in Si‐doped boron carbide, and (3) calibration of a scanning electron microscope X‐ray energy‐dispersive spectroscopy (XEDS) system to measure compositional homogeneity differences of B/Si‐doped arc‐melted boron carbides in the as‐melted and annealed conditions. Overall, the improvement and application of advanced analytical tools have helped better understand processing–microstructure–property relationships and successfully manufacture high‐performance ceramics.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jul 30, 2021
Source ID
10.1111/jace.18039

Entities

People

  • Christopher J. Marvel
  • Jerry C LaSalvia
  • Kristopher D. Behler
  • Martin P Harmer
  • Masashi Watanabe
  • Qirong Yang
  • Richard A Haber
  • Scott D. Walck
  • Yuxuan Xie

Organizations

  • Lawrence Livermore National Laboratory
  • Lehigh University
  • Rutgers University
  • United States Army Research Laboratory

Tags

Readers

  • Computational Modeling and Simulation
  • Distributed Systems and Data Platform Development
  • Powder metallurgy of Titanium alloys.

Technology Areas

  • Microelectronics