Photochemical Immobilization of Polymers on a Surface: Controlling Film Thickness and Wettability

Abstract

In this manuscript, we demonstrate the control of film thickness and surface wettability in the photochemical immobilization of poly (vinyl alcohol) (PVA) to a self‐assembled monolayer (SAM) containing a phthalimide chromophore. Surface attachment is characterized by ellipsometry and contact angle measurements. The wettability of the resulting films is shown to depend on the chemical composition of the polymer. The film thickness is shown to depend on the irradiation time and molecular weight of the polymer. Using a photomask, micropatterns of polymers can be grafted to the SAM. The photopatterned surface can be “developed” by coating with a thin layer of a mixture containing poly (styrene) (PS) and triphenylsulfonium triflate.

Document Details

Document Type
Pub Defense Publication
Publication Date
Apr 27, 2017
Source ID
10.1111/php.12751

Entities

People

  • Angela Mammana
  • Gregory T. Carroll
  • Jeffrey T Koberstein
  • Nicholas J. Turro

Organizations

  • Columbia University
  • Empire State Development Division of Science, Technology and Innovation
  • National Science Foundation
  • United States Army
  • United States Army Research Laboratory
  • University of Dayton

Tags

Fields of Study

  • Materials science

Readers

  • Nanofabrication and Microfabrication.
  • Organic Chemistry
  • Surface Coatings Technology.