Uniform sputter deposition of high-quality epitaxial complex oxide thin films

Abstract

Uniform deposition of high-quality epitaxial complex oxide thin films over a large area is desirable not only for the large scale fabrication of oxide electronics but also for preparing multiple samples with the same growth conditions for various characterization techniques. However, it is particularly challenging to grow uniform thin films of multicomponent oxide systems containing volatile species such as Pb and Bi. By combining a misaligned parallel dual planar magnetron sputtering technique with substrate rotation, the authors have grown uniform epitaxial thin films piezoelectric 0.67Pb(Mg1/3Nb2/3)O3–0.33PbTiO3 and multiferroic monodomain BiFeO3 with high-deposition rates over a 2 in. diameter area. These films have excellent uniformity of thickness, stoichiometric compositions, and electrical properties. This technique can be scaled to larger deposition areas by using larger sputtering targets and widely applied to various multicomponent complex oxide thin film heterostructures.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 05, 2017
Source ID
10.1116/1.4998956

Entities

People

  • A. Brewer
  • C. B. Eom
  • J. C. Frederick
  • K. H. Cho
  • S. H. Baek
  • Wittawat Saenrang

Organizations

  • Army Research Office
  • National Science Foundation
  • University of Wisconsin–Madison

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Nanofabrication and Microfabrication.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene