Electronic structure of BaSnO3 investigated by high-energy-resolution electron energy-loss spectroscopy and ab initio calculations

Abstract

There has been growing interest in perovskite BaSnO3 due to its desirable properties for oxide electronic devices, including high electron mobility at room temperature and optical transparency. As these electronic and optical properties originate largely from the electronic structure of the material, here the basic electronic structure of epitaxially grown BaSnO3 films is studied using high-energy-resolution electron energy-loss spectroscopy in a transmission electron microscope and ab initio calculations. This study provides a detailed description of the dielectric function of BaSnO3, including the energies of bulk plasmon excitations and critical interband electronic transitions, the band structure and partial densities of states, the measured band gap, and more.

Document Details

Document Type
Pub Defense Publication
Publication Date
Mar 12, 2018
Source ID
10.1116/1.5026298

Entities

People

  • Abhinav Prakash
  • Bharat Jalan
  • Chris Leighton
  • Hwanhui Yun
  • Jong Seok Jeong
  • K. Andre Mkhoyan
  • Koustav Ganguly
  • Mehmet Topsakal
  • Renata M. Wentzcovitch

Organizations

  • Defense Threat Reduction Agency
  • National Science Foundation
  • University of Minnesota

Tags

Fields of Study

  • Materials science
  • Physics

Readers

  • Marine Hydrodynamics
  • Quantum Chemistry
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene