Growth and characterization of α-Ga2O3 on sapphire and nanocrystalline β-Ga2O3 on diamond substrates by halide vapor phase epitaxy

Abstract

Halide vapor phase epitaxial (HVPE) Ga2O3 films were grown on c-plane sapphire and diamond substrates at temperatures up to 550 °C without the use of a barrier dielectric layer to protect the diamond surface. Corundum phase α-Ga2O3 was grown on the sapphire substrates, whereas the growth on diamond resulted in regions of nanocrystalline β-Ga2O3 (nc-β-Ga2O3) when oxygen was present in the HVPE reactor only during film growth. X-ray diffraction confirmed the growth of α-Ga2O3 on sapphire but failed to detect any β-Ga2O3 reflections from the films grown on diamond. These films were further characterized via Raman spectroscopy, which revealed the β-Ga2O3 phase of these films. Transmission electron microscopy demonstrated the nanocrystalline character of these films. From cathodoluminescence spectra, three emission bands, UVL′, UVL, and BL, were observed for both the α-Ga2O3/sapphire and nc-Ga2O3/diamond, and these bands were centered at approximately 3.7, 3.2, and 2.7 eV.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 03, 2022
Source ID
10.1116/6.0002115

Entities

People

  • Akito Kuramata
  • Aman Haque
  • James Spencer Lundh
  • Leonid Chernyak
  • Marko J. Tadjer
  • Nahid Sultan Al-Mamun
  • Stephen Pearton
  • Sushrut Modak
  • Thieu Quang Tu

Organizations

  • Defense Threat Reduction Agency
  • NATO
  • National Research Council
  • National Science Foundation
  • Pennsylvania State University
  • United States Naval Research Laboratory
  • United States – Israel Binational Science Foundation
  • University of Central Florida
  • University of Florida

Tags

Fields of Study

  • Materials science

Readers

  • Semiconductor Device Technology
  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene