Direct observation of triplet energy transfer from semiconductor nanocrystals

Abstract

Most molecules adopt a singlet spin configuration: All their electrons are arranged in pairs. Unpaired triplet states engage in a variety of useful reactions but are hard to produce. Quantum mechanics dictates that photo-excitation from singlet to triplet states is inefficient. Instead, chemists rely on sensitizers, which populate the triplet states of their neighbors through energy transfer after absorbing light themselves. Mongin et al. now show that certain nanoparticles can act as triplet sensitizers.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 22, 2016
Source ID
10.1126/science.aad6378

Entities

People

  • Cédric Mongin
  • Felix Castellano
  • Mikhail Zamkov
  • Natalia Razgoniaeva
  • Sofia Garakyaraghi

Organizations

  • Air Force Office of Scientific Research
  • Argonne National Laboratory
  • Bowling Green State University
  • National Science Foundation
  • North Carolina State University

Tags

Fields of Study

  • Chemistry
  • Physics

Readers

  • Molecular Genetics
  • Nanocomposite Materials Science
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Biotechnology
  • Microelectronics
  • Quantum Computing