Single-particle mapping of nonequilibrium nanocrystal transformations

Abstract

The control of the shape and size of metal nanoparticles can be very sensitive to the growth conditions of the particles. Ye et al. studied the reverse process: They tracked the dissolution of gold nanoparticles in a redox environment inside a liquid cell within an electron microscope, controlling the particle dissolution with the electron beam. Tracking short-lived particle shapes revealed structures of greater or lesser stability. The findings suggest kinetic routes to particle sizes and shapes that would otherwise be difficult to generate.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 18, 2016
Source ID
10.1126/science.aah4434

Entities

People

  • Alex Zettl
  • Alexander S. Powers
  • Eran Rabani
  • Gabriel Dunn
  • Grant M. Rotskoff
  • Layne B. Frechette
  • Matthew R. Jones
  • Paul Alivisatos
  • Peter Ercius
  • Phillip L. Geissler
  • Qian Chen
  • Son C. Nguyen
  • Vivekananda P Adiga
  • Xingchen Ye

Organizations

  • Arnold and Mabel Beckman Foundation
  • Bulgarian Science Fund
  • Defense Threat Reduction Agency
  • King Abdulaziz City for Science and Technology
  • Lawrence Berkeley National Laboratory
  • Miller Institute
  • National Science Foundation
  • Tel Aviv University
  • United States Department of Energy
  • University of California, Berkeley
  • Yusuf Hamied Department of Chemistry

Tags

Fields of Study

  • Physics

Readers

  • Brain and Cognitive Science; Experimental Psychology; Cognitive Neuroscience
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Nanoscale Plasmonic Nanotechnology

Technology Areas

  • Biotechnology
  • Directed Energy
  • Microelectronics