Semiconducting polymer blends that exhibit stable charge transport at high temperatures

Abstract

Charge carriers move through semiconductor polymers by hopping transport. In principle, these polymers should be more conductive at higher temperatures. In practice, conductivity drops at high temperatures because interchain contacts are disrupted, which limits potential applications. Gumyusenge et al. now show that appropriate blending of a semicrystalline conjugated polymer with an insulating polymer that has a high glass-transition temperature creates a morphology that stabilizes a network of semiconductor channels. High charge conductivity was maintained in these materials up to 220°C.

Document Details

Document Type
Pub Defense Publication
Publication Date
Dec 07, 2018
Source ID
10.1126/science.aau0759

Entities

People

  • Alexander L Ayzner
  • Aristide Gumyusenge
  • Brett Savoie
  • Dung T. Tran
  • Gregory M. Pitch
  • Jianguo Mei
  • Kaelon A. Jenkins
  • Tim J. Dunn
  • Xuyi Luo
  • Yan Zhao

Organizations

  • National Science Foundation
  • Office of Naval Research
  • Purdue University
  • Stanford University
  • University of California, Santa Cruz

Tags

Fields of Study

  • Materials science

Readers

  • Materials Science and Engineering.
  • Quantum Chemistry
  • Thermal Physics or Thermal Science.

Technology Areas

  • Microelectronics