Solvation sheath reorganization enables divalent metal batteries with fast interfacial charge transfer kinetics

Abstract

Divalent rechargeable metal batteries such as those based on magnesium and calcium are of interest because of the abundance of these elements and their lower tendency to form dendrites, but practical demonstrations are lacking. Hou et al . used methoxyethyl amine chelants in which the ligands attach to the metal atom in more than one place, modulating the solvation structure of the metal ions to enable a facile charge-transfer reaction (see the Perspective by Zuo and Yin). In full battery cells, these components lead to high efficiency and energy density. Theoretical calculations were used to understand the solvation structures. —MSL

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 08, 2021
Source ID
10.1126/science.abg3954

Entities

People

  • Chunsheng Wang
  • Jijian Xu
  • Karen J. Gaskell
  • Luning Wang
  • Oleg Borodin
  • Peng-Fei Wang
  • Ruimin Sun
  • Singyuk Hou
  • Xiao Ji

Organizations

  • United States Army Combat Capabilities Development Command
  • University of Maryland

Tags

Fields of Study

  • Chemistry

Readers

  • Battery Technology and Engineering
  • Marine Mammal Biology
  • Quantum Chemistry