A Bayesian Approach to Autonomous Analysis of Electrochemical Impedance Spectra

Abstract

Electrochemical impedance spectroscopy (EIS) is a valuable characterization tool for a wide variety of materials due to its ability to probe transport and reaction pathways over a broad range of timescales. Recently, developments in experimental techniques have increased the use of EIS in high-throughput materials characterization. However, extraction of meaningful insight from high-volume EIS data streams is often stymied by the complexity of processing and analyzing impedance spectra. To address this challenge, we present a framework for fully autonomous analysis of EIS data leveraging Bayesian methods to obtain both the distribution of relaxation times (DRT) and equivalent circuit fits.

Document Details

Document Type
Pub Defense Publication
Publication Date
Nov 23, 2020
Source ID
10.1149/ma2020-02402508mtgabs

Entities

People

  • Andriy Zakutayev
  • Jake Huang
  • Meagan C Papac
  • Ryan O'Hayre

Tags

Readers

  • Analytical Chemistry
  • Distributed Systems and Data Platform Development
  • Environmental Impact Assessment (EIA) of Proposed Air Force Base Actions.

Technology Areas

  • AI & ML
  • AI & ML - Bayesian Inference