AnIn VitroComparison of PMMA and Calcium Sulfate as Carriers for the Local Delivery of Gallium(III) Nitrate to Staphylococcal Infected Surgical Sites

Abstract

Antibiotic-loaded bone cements, including poly(methyl methacrylate) (PMMA) and calcium sulfate (CaSO4), are often used for treatment of orthopaedic infections involvingStaphylococcusspp., although the effectiveness of this treatment modality may be limited due to the emergence of antimicrobial resistance and/or the development of biofilms within surgical sites. Gallium(III) is an iron analog capable of inhibiting essential iron-dependent pathways, exerting broad antimicrobial activity against multiple microorganisms, includingStaphylococcusspp. Herein, we evaluated PMMA and CaSO4as carriers for delivery of gallium(III) nitrate (Ga(NO3)3) to infected surgical sites by assessing the release kinetics subsequent to incorporation and antimicrobial activity againstS. aureusandS. epidermidis. PMMA and to a lesser extent CaSO4were observed to be compatible as carriers for Ga(NO3)3, eluting concentrations with antimicrobial activity against planktonic bacteria, inhibiting bacterial growth, and preventing bacterial colonization of beads, and effective against established bacterial biofilms ofS. aureusandS. epidermidis. Collectively, ourin vitroresults indicate that PMMA is a more suitable carrier compared to CaSO4for delivery of Ga(NO3)3; moreover they provide evidence for the potential use of Ga(NO3)3with PMMA as a strategy for the prevention and/or treatment for orthopaedic infections.

Document Details

Document Type
Pub Defense Publication
Publication Date
Jan 01, 2016
Source ID
10.1155/2016/7078989

Entities

People

  • Carlos J. Sanchez
  • David Chang
  • David J. Tennent
  • Joseph C Wenke
  • Rebecca A. Garcia

Organizations

  • United States Army Medical Research and Development Command

Tags

Fields of Study

  • Materials science

Readers

  • Molecular and Cellular Biochemistry
  • Polymer Science and Technology
  • Trauma Surgery or Emergency Medicine.

Technology Areas

  • Biotechnology
  • Microelectronics