Flexible random lasers in dye-doped bio-degradable cellulose nanocrystalline needles

Abstract

In this work, we developed and investigated a random laser based on rhodamine6G (Rh6G) in ethylene glycol (EG) solution with varying cellulose nanocrystalline (CNC) needles as scatterers in the lasing media. Besides the suspension-in-cuvette scheme, an alternative configuration was also employed: a dye-CNC flexible self-supported thick-film (70 µm) random laser made by drop casting of the C N C s + R h 6 G + h y d r o x y p r o p y l cellulose suspension. In relation to conventional scatterers, the biodegradable cellulose nanocompounds showed a comparable reduction in both the spectral full width at half-maximum and the energy threshold values, with an optimal concentration of 5 mg [CNC]/ml[EG] in suspension. Its performance was also compared with other cellulose-based random lasers, presenting advantages for some parameters. The flexible film configuration showed similar results, but contained 10% less Rh6G than the suspension.

Document Details

Document Type
Pub Defense Publication
Publication Date
Dec 04, 2019
Source ID
10.1364/josab.37.000024

Entities

People

  • Anderson S. L. Gomes
  • Antonio Mario L. M. Costa
  • Edison Pecoraro
  • Gleice C. M. Germano
  • Isabel Cristina dos Santos Carvalho
  • Lucas Martinho
  • Susete N. Fernandes
  • Yan D. R. Machado

Organizations

  • Coordenação de Aperfeicoamento de Pessoal de Nível Superior
  • European Regional Development Fund
  • Financiadora de Estudos e Projetos
  • Fundação de Amparo à Ciência e Tecnologia de Pernambuco
  • Fundação para a Ciência e Tecnologia
  • National Council for Scientific and Technological Development
  • Office of Naval Research Global

Tags

Fields of Study

  • Materials science

Readers

  • Optical Physics and Photonics.
  • Polymer Science and Engineering.
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition