Highly sensitive detection of broadband terahertz waves using aqueous salt solutions
Abstract
Water-based coherent detection of broadband terahertz (THz) wave has been recently proposed with superior performances, which can alleviate the limited detection bandwidth and high probe laser energy requirement in the solid- and air-based detection schemes, respectively. Here, we demonstrate that the water-based detection method can be extended to the aqueous salt solutions and the sensitivity can be significantly enhanced. The THz coherent detection signal intensity scales linearly with the third-order nonlinear susceptibility χ(3) or quadratically with the linear refractive index η0 of the aqueous salt solutions, while the incoherent detection signal intensity scales quadratically with χ(3) or quartically with η0, proving the underlying mechanism is the four-wave mixing. Both the coherent and incoherent detection signal intensities appear positive correlation with the solution concentration. These results imply that the liquid-based THz detection scheme could provide a new technique to measure χ(3) and further investigate the physicochemical properties in the THz band for various liquids.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Oct 07, 2022
- Source ID
- 10.1364/oe.472753
Entities
People
- Cun-lin Zhang
- Liangliang Zhang
- Ming-hao Zhang
- Rui Zhang
- Wei-Min Wang
- Wen Xiao
- Xi-Cheng Zhang
Organizations
- Air Force Office of Scientific Research
- Capital Normal University
- National Natural Science Foundation of China
- National Science Foundation
- Renmin University of China
- Shanghai Jiao Tong University
- University of Rochester