Terahertz nonlinear index extraction via full-phase analysis

Abstract

We experimentally show the spectrally averaged nonlinear refractive index and absorption coefficient for liquid water, water vapor, α -pinene, and Si using a full-phase analysis in the terahertz regime through a standard time-domain spectrometer. Our results confirm that the nonlinear index of refraction of the liquid samples in this regime exceeds the near-infrared optical nonlinear index by six orders of magnitude. In the case of liquid water and water vapor at atmospheric pressure, we find a nonlinear index of 7.8 × 10 − 10 c m 2 / W and 6 × 10 − 11 c m 2 / W , respectively, which are both much larger than expected.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 07, 2020
Source ID
10.1364/ol.399999

Entities

People

  • Kareem J. Garriga Francis
  • Mervin Lim Pac Chong
  • X.-C. Zhang
  • Yiwen E

Organizations

  • Air Force Office of Scientific Research
  • Army Research Office
  • Gates Foundation
  • National Science Foundation

Tags

Fields of Study

  • Physics

Readers

  • Aerosol Science/Aerosol Physics
  • Control Systems Engineering.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.