Copolyimides for gradient-index optics

Abstract

Copolymerization offers a promising route to the accurate control of material properties, such as refractive index. For compatible polymers, an ability to produce copolymers with incrementally varying refractive indices is a basic requirement for fabricating gradient-index (GRIN) optics. To determine the accuracy of this approach, we examined the composition dependence of index in several optical copolyimides. We observed deviations from standard model predictions that exceed 5 × 10−3 at certain compositions, consistent with non-ideal copolymer formation. This implies that state-of-the-art GRIN optical design requires careful calibration of the composition dependence in these copolymers. We further found that birefringence is sensitive to the structures of the component polymers, and that the thermo-optic and thermal expansion coefficients vary linearly with composition, within the experimental uncertainty.

Document Details

Document Type
Pub Defense Publication
Publication Date
Sep 23, 2022
Source ID
10.1364/ome.460831

Entities

People

  • Armand Rosenberg
  • James S. Shirk
  • Sang Ho Lee

Organizations

  • Office of Naval Research
  • United States Naval Research Laboratory

Tags

Fields of Study

  • Physics

Readers

  • Combustion science or combustion engineering.
  • Optical Physics and Photonics.
  • Polymer Science and Engineering.

Technology Areas

  • Microelectronics