Photoluminescence microscopy as a noninvasive characterization method for defects in gallium oxide and aluminum gallium oxide epitaxial films

Abstract

Herein we utilize polarized photoluminescence (PL) microscopy and spectral analysis to locate and characterize many different types of µm-scale extended defects present in melt-grown bulk crystals and metal-organic vapor-phase epitaxy (MOVPE)-grown epitaxial thin films of β-Ga2O3 and β-(Al,Ga)2O3. These include pits, divots, mounds, scratches, rotation domain boundaries, stacking faults, cracks, and other defect categories. Some types of µm-scale defects simply decrease overall PL yield, while others emit different spectra than single crystal regions. We combine PL microscopy with atomic force microscopy (AFM) and scanning electron microscopy (SEM) to provide detailed characteristics of these different types of features which can arise from both bulk crystal growth, surface preparation, and epitaxial growth processes. We show that sample quality (in terms of extended defects) can be determined by using PL and that attributing spectral features to isolated point defects is invalid unless the sample is proven to not contain extended defects.

Document Details

Document Type
Pub Defense Publication
Publication Date
Oct 13, 2022
Source ID
10.1364/ome.474921

Entities

People

  • Arkka Bhattacharyya
  • Berardi Sensale-Rodriguez
  • Jacqueline Cooke
  • Jani Jesenovec
  • John S. McCloy
  • Michael A. Scarpulla
  • Praneeth Ranga
  • Sriram Krishnamoorthy
  • Xueling Cheng
  • Yunshan Wang

Organizations

  • Air Force Office of Scientific Research
  • University of California
  • University of Utah
  • Washington State University

Tags

Fields of Study

  • Materials science

Readers

  • Nanoscale Plasmonic Nanotechnology
  • Semiconductor Device Technology
  • Thin Film Deposition Science.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene