Strain tuning of the emission axis of quantum emitters in an atomically thin semiconductor

Abstract

Strain engineering is a natural route to control the electronic and optical properties of two-dimensional (2D) materials. Recently, 2D semiconductors have also been demonstrated as an intriguing host of strain-induced quantum-confined emitters with unique valley properties inherited from the host semiconductor. Here, we study the continuous and reversible tuning of the light emitted by such localized emitters in a monolayer tungsten diselenide embedded in a van der Waals heterostructure. Biaxial strain is applied on the emitters via strain transfer from a lead magnesium niobate–lead titanate (PMN-PT) piezoelectric substrate. Efficient modulation of the emission energy of several localized emitters up to 10 meV has been demonstrated on application of a voltage on the piezoelectric substrate. Further, we also find that the emission axis rotates by ∼ 40 ∘ as the magnitude of the biaxial strain is varied on these emitters. These results elevate the prospect of using all electrically controlled devices where the property of the localized emitters in a 2D host can be engineered with elastic fields for an integrated opto-electronics and nano-photonics platform.

Document Details

Document Type
Pub Defense Publication
Publication Date
May 27, 2020
Source ID
10.1364/optica.377886

Entities

People

  • Arunabh Mukherjee
  • Carla Watson
  • Chitraleema Chakraborty
  • Dirk Englund
  • Hyowon Moon
  • Kumarasiri Konthasinghe
  • Liangyu Qiu
  • Nick Vamivakas
  • Stephen M. Wu
  • Tara Peña
  • Wenhui Hou

Organizations

  • Air Force Office of Scientific Research
  • Army Research Office
  • National Science Foundation
  • National Science Foundation Directorate for Mathematical & Physical Sciences

Tags

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Quantum Dot Semiconductor Device Photonics and Graphene Optoelectronic Materials and THz Physics.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene
  • Quantum Computing