Broad Frequency Shift of Parametric Processes in Epsilon-Near-Zero Time-Varying Media

Abstract

The ultrafast changes of material properties induced by short laser pulses can lead to a frequency shift of reflected and transmitted radiation. Recent reports highlight how such a frequency shift is enhanced in spectral regions where the material features a near-zero real part of the permittivity. Here, we investigate the frequency shift for fields generated by four-wave mixing. In our experiment, we observed a frequency shift of more than 60 nm (compared to the pulse width of ∼40 nm) in the phase conjugated radiation generated by a 500 nm aluminium-doped zinc oxide (AZO) film pumped close to the epsilon-near-zero wavelength. Our results indicate applications of time-varying media for nonlinear optics and frequency conversion.

Document Details

Document Type
Pub Defense Publication
Publication Date
Feb 15, 2020
Source ID
10.3390/app10041318

Entities

People

  • Alexandra Boltasseva
  • Clayton Devault
  • Daniele Faccio
  • Enrico Carnemolla
  • Marcello Ferrera
  • Matteo Clerici
  • Stefano Vezzoli
  • Vincenzo Bruno
  • Vladimir M. Shalaev

Organizations

  • Air Force Office of Scientific Research
  • Engineering and Physical Sciences Research Council
  • Office of Naval Research
  • Savannah River Operations Office
  • UK Research and Innovation

Tags

Fields of Study

  • Physics

Readers

  • Nanofabrication and Microfabrication.
  • Optical Physics and Photonics.
  • Polymer Science and Technology

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Directed Energy - Pulsed-Laser Deposition