Intensity-Dependent Optical Response of 2D LTMDs Suspensions: From Thermal to Electronic Nonlinearities
Abstract
The nonlinear optical (NLO) response of photonic materials plays an important role in the understanding of light–matter interaction as well as pointing out a diversity of photonic and optoelectronic applications. Among the recently studied materials, 2D-LTMDs (bi-dimensional layered transition metal dichalcogenides) have appeared as a beyond-graphene nanomaterial with semiconducting and metallic optical properties. In this article, we review most of our work in studies of the NLO response of a series of 2D-LTMDs nanomaterials in suspension, using six different NLO techniques, namely hyper Rayleigh scattering, Z-scan, photoacoustic Z-scan, optical Kerr gate, and spatial self-phase modulation, besides the Fourier transform nonlinear optics technique, to infer the nonlinear optical response of semiconducting MoS2, MoSe2, MoTe2, WS2, semimetallic WTe2, ZrTe2, and metallic NbS2 and NbSe2. The nonlinear optical response from a thermal to non-thermal origin was studied, and the nonlinear refraction index and nonlinear absorption coefficient, where present, were measured. Theoretical support was given to explain the origin of the nonlinear responses, which is very dependent on the spectro-temporal regime of the optical source employed in the studies.
Document Details
- Document Type
- Pub Defense Publication
- Publication Date
- Aug 07, 2023
- Source ID
- 10.3390/nano13152267
Entities
People
- Ali M. Jawaid
- Anderson Stevens Leonidas Gomes
- Cecília L. A. V. Campos
- Cid Bartolomeu de Araújo
- Manoel L da Silva-Neto
- Melissa Maldonado
- Richard A. Vaia
- Robert Busch
Organizations
- Air Force Office of Scientific Research
- Air Force Research Laboratory
- Coordenação de Aperfeicoamento de Pessoal de Nível Superior
- Institute of Physics