ELECTRON COUPLING OF PROTON SPINS IN HETEROCYCLIC MOLECULES. N-BENZYLTHIENO 3,2-B PYRROLE

Abstract

THE HIGH-RESOLUTION PROTON MAGNETIC RESONANCE SPECTRUM OF THE FOUR PROTONS ATTACHED TO THE HETEROCYCLIC RINGS OF N-BENZYLTHIENO 3,2-B PYRROLE (I) HAS BEEN EXAMINED. THE SPECTRUM IS OF THE TYPE ABCD PERTURBED BY TWO NUCLEI X2 WHICH COUPLE WITH A, AND IT INVOLVES THREE LONG-RANGE PROTON-PROTON COUPLINGS, 0.5, 1.3 AND 0.3 CPS OVER FIVE, SIX, AND SIX BONDS RESPECTIVELY, WHICH CAN BE ACCOUNTED FOR ONLY BY PI ELECTRON INTERACTIONS. THE COUPLING CONSTANTS FOUND IN EACH OF THE RINGS IN I ARE COMPARED WITH THOSE FOR THIOPHENE AND PYRROLE. ANGULAR EFFECTS AS WELL AS ELECTRONEGATIVITY DIFFERENCES GOVERN THE COUPLING VIA SIGMA ELECTRONS IN HCCH GROUPS

Document Details

Document Type
Technical Report
Publication Date
Dec 29, 1961
Accession Number
AD0250681

Entities

People

  • A.l. Porte
  • Herbert S. Gutowsky

Organizations

  • University of Illinois Urbana–Champaign

Tags

DTIC Thesaurus Topics

  • Coupling (Interaction)
  • Couplings
  • Electrons
  • High Resolution
  • Magnetic Resonance
  • Molecules
  • Motion
  • Resonance
  • Spectra

Fields of Study

  • Chemistry
  • Physics

Readers

  • Quantum Chemistry
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Microelectronics