Radiochemical Determination of Sodium-24 and Sulfur-35 in Seawater

Abstract

Rapid radiochemical procedures were developed for determining Na24 and S35 in seawater containing fission product radionuclides. Na24 is separated from other radionuclides by scavenging with lanthanum hydroxide; two NaCe precipitations with HCl gas follow. The disintegration rate is determined by measuring the area of the 1.368 Mev gamma photopeak. The working time required for a single analysis is 1/2 hr; the precision, plus or minus 1 percent; the chemical yield, about 70 percent; and the total effective decontamination factor from fission products greater than 100,000. S35 in seawater is separated from other radionuclides through precipitating BaSO4. This is followed by reducing the sulfate to H2S with HI and by subsequently oxidizing sulfide to sulfate in an alkaline peroxide solution. The resulting sulfate ion is precipitated as BaSO4 for chemical yield determination and counting. The working time required for a single analysis is less than 1 hr; the precision, plus or minus 5 percent; the chemical yield, 70-80 percent; and the decontamination factor from fission products, greater than 10 to the 7th power.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jul 10, 1961
Accession Number
AD0262444

Entities

People

  • D. Love
  • D. Sam

Organizations

  • Naval Radiological Defense Laboratory

Tags

Communities of Interest

  • Air Platforms
  • Biomedical
  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Barium Compounds
  • Chemical Synthesis
  • Chemistry
  • Dielectric Gases
  • Filter Paper
  • Fission Products
  • Gamma Rays
  • Hydrochloric Acid
  • Hydrogen
  • Materials
  • Measurement
  • Physical Chemistry
  • Precipitation
  • Radiation Measuring Instruments
  • Sodium Compounds
  • Spectrometers
  • Standards

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Environmental Engineering
  • Solar Physics