TETRAKIS (P-DIMETHYLAMINOPHENYL) ETHYLENE DIIODIDE AND ITS FREE RADICAL BEHAVIOR

Abstract

Tetrakis-(p-dimethylaminophenyl) ethylene (I) was shaken with AgNO3 in water for 12 hr to produce two dinitrate derivative (II); addition of KI to II in water produced two diiodide derivative (III), brilliant green crystals precipitated from water. Water solutions of II and III showed no E.P.R. signal. In ethylene chloride there was a marked difference between the optical and E.P.R. spectra of II and III. Solutions of II were purple and showed no radical activity; solutions of III were green ang gave an intense E.P.R. signal, corresponding to at least 20% of the material being a free radical. The optical and E.P.R. spectra are the same whether III is dissolved in ethylene chloride or iodine is added to I in ethylene chloride.

Document Details

Document Type
Technical Report
Publication Date
Jul 23, 1961
Accession Number
AD0263173

Entities

People

  • D.h. Anderson
  • R.m. Elofson

Organizations

  • University of Illinois Urbana–Champaign

Tags

DTIC Thesaurus Topics

  • Acyclic Hydrocarbons
  • Alkenes
  • Chemical Compounds
  • Chlorides
  • Ethylenes
  • Free Radicals
  • Hydrocarbons
  • Materials
  • Organic Compounds
  • Spectra

Fields of Study

  • Chemistry

Readers

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  • Materials Science and Engineering.
  • Organic Chemistry