THE OXYGEN ELECTRODE IN FUSED ELECTROLYTES

Abstract

The Pt/O2 electrode system is evaluated in a molten carbonate electrolyte at 600 - 800 C by the criteria for reference electrodes. This electrode system is found to be stable and reproducible (+ or - 5 mv) and shows a high degree of reversibility by the criteria of bias-potentials, micropolarization, and the Nernst Equation. It is apparent that this electrode system functions as a relative of the metalmetal xide class of reference electrodes. Some results are also reported for gold, rather than platinum, as the metal substrate. While the Au/O2 system satisfies the above criteria for reference electrodes, there is evidence that it equilibrates at/an energy state slightly higher in thermodynamic free energy than the Pt/O2 system. (Author)

Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1961
Accession Number
AD0263953

Entities

People

  • Fumihiko Saegusa
  • George J. Janz

Organizations

  • Rensselaer Polytechnic Institute

Tags

DTIC Thesaurus Topics

  • Carbonates
  • Chemical Compounds
  • Electrical Equipment
  • Electrodes
  • Electrolytes
  • Energy
  • Equations
  • Free Energy
  • Metals
  • Oxygen Electrodes
  • Platinum
  • Substrates

Fields of Study

  • Materials science

Readers

  • Adaptive Control and Estimation with Uncertainty in Dynamic Systems.
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Linear Algebra