RESEARCH ON LOW TEMPERATURE FUEL CELL SYSTEMS
Abstract
The polarization behavior of the oxygen electrode or hydrogen-oxygen cells on open circuit and in the non-linear region is shown to depend, among other factors, on (a) type of electrode material (b) surface treatment (c) pH (d) presence of foreign ions and their concentrations (e) stirring or agitation (f) cell design parameters and the technique of single electrode potential measurement. Most significant experimental observations concerning the open circuit behavior include (a) transient open circuit voltages greater than the thermodynamically reversible potential of 1.23 volts under certain conditions, (b) experimentally observed effect of higher temperature on the open circuit voltage of the oxygen electrode is in a direction opposite to thermodynamic predictions. Experimental evidence is presented to show that the hydrogen and oxygen electrodes operating in the same bulk electrolyte under steady-state current flow conditions are always associated with significant pH changes (or concentration gradient) at each electrode. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Aug 15, 1961
- Accession Number
- AD0265763
Entities
Organizations
- General Electric