CHEMISTRY OF DECABORANE PHOSPHORUS COMPOUNDS. II. SYNTHESIS AND REACTIONS OF DIPHENYLPHOSPHINODECABORANE

Abstract

Decaboranyl sodium and diphenylchlorophosphine reacted in ether solution to form diphenylphosphinodecaborane (Ph2P-B10H13), the first phosphine substituted decaborane with trivalent phosphorus. B-11 NMR spectral investigation proved the substituent to be at the 6-position. Unlike monomeric phosphinoboranes (R2P-BR2), it is unreactive toward Lewis acids, oxidation and quaternization, but undergoes partial degradation with alcohols to form B9H13-(Ph2PH). Its reactions with amines and phosphines resulting in salts containing the Ph2PB10H12 anion are described. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jul 26, 1962
Accession Number
AD0278702

Entities

People

  • Hansjuergen Schroeder

Tags

DTIC Thesaurus Topics

  • Acids
  • Chemical Compounds
  • Chemical Synthesis
  • Chemistry
  • Degradation
  • Lewis Acids
  • Organophosphorus Compounds
  • Oxidation
  • Phosphine
  • Phosphorus
  • Phosphorus Compounds

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry