THERMOELECTRIC INSTABILITY OF SOME NOBLE METAL THERMOCOUPLES AT HIGH TEMPERATURES

Abstract

Thermoelectric instabilities of noble metal thermocouples and individual thermoelements were studied from 1000 to 1700 deg C under oxidizing and neutral atmospheres. The principal source of instability was a contamination of the thermoelements by impurities from ceramic protection tubes. Several grades of alumina sheathing were tested, and thermocouple errors associated with each grade were determined. With alumina sheathing the principal contaminant was iron, and the instability generated was at least an order of magnitude greater in a neutral atmosphere than in an oxidizing atmosphere. Increasing the wire size increases stability in a neutral atmosphere, although not in an oxidizing atmosphere. Instability increases rapidly with temperature between 1000 and 1700 deg C, but the order of decreasing stability remains Pt-6%Rh/Pt-30%Rh, Pt-1%Rh/Pt-13%Rh, and Pt/Pt-10%Rh or Pt/Pt-13%Rh. The instability of pure rhodium thermoelements, and of Ir and Ir-50%Rh thermoelements, depends on internal changes, and not as much on iron contamination as the Pt-Rh series of thermoelements; hence the pure rhodium and the iridium thermoelements become preferable if gross iron contamination is expected.

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Document Details

Document Type
Technical Report
Publication Date
Jun 29, 1962
Accession Number
AD0282154

Entities

People

  • B. E. Walker
  • C. T. Ewing
  • Roman R. Miller

Organizations

  • United States Naval Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Chemical Analysis
  • Chemical Synthesis
  • Chemistry
  • Elements
  • Geometry
  • High Temperature
  • Iron Compounds
  • Materials
  • Materials Science
  • Measurement
  • Melting Point
  • Metals
  • Military Research
  • Reliability
  • Rhodium Alloys
  • Standards
  • Temperature Gradients

Fields of Study

  • Materials science

Readers

  • Surface Engineering/Surface Coating Technology.
  • Thermal Physics or Thermal Science.