KINETICS OF RECOMBINATION PROCESSES

Abstract

Rate coefficients for formation of N2, NO, H2, HO2, H2O2, He2(+), and Ar2(+) from atoms, atomic ions, or free radicals in triple collisions were measured at 300 K. A theoretical evaluation of the rate coefficient for diatomic molecule formation in triple collisions was carried out, giving results which agreed well with the experimental values. Rate coefficients for several bimolecular reactions involving O atoms, N atoms, or OH radicals were also determined. A theory of positive ion collection by Langmuir probes in gas discharge plasmas at pressures between about 0.1 and 20 mm Hg was developed. Dissociative recombination coefficients of Ar, N, O, Hg, and Cs molecular ions were determined from probe measurements on gas discharge afterglows, using this theory to calculate ion concentrations from probe currents. Recombination coefficients obtained in this manner agreed well with values obtained by microwave techniques. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jun 14, 1962
Accession Number
AD0283043

Entities

People

  • C.b. Kretschmer

Organizations

  • Aerojet Rocketdyne Holdings

Tags

DTIC Thesaurus Topics

  • Afterglows
  • Chemical Reactions
  • Coefficients
  • Collisions
  • Diatomic Molecules
  • Free Radicals
  • Gas Discharges
  • Kinetics
  • Langmuir Probes
  • Measurement
  • Microwaves
  • Molecules
  • Probes
  • Test And Evaluation

Readers

  • Materials Science and Engineering.
  • Pulsed Power and Plasma Physics.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.