NATURAL EXPANSION OF EXACT WAVE FUNCTIONS. II. THE HYDROGEN MOLECULE GROUND STATE
Abstract
The Kolos and Roothaan wave function for H2 has been analyzed into natural orbitals. It was found that the first natural orbital is nearly the SCF function. The first four natural orbitals provide a good description of the molecule and give a total energy of -1.169884 Hartrees. Beyond the first four terms, the natural expansion becomes more slowly convergent. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Jul 03, 1962
- Accession Number
- AD0283426
Entities
People
- Ernest R. Davidson
- Leon L. Jones
Organizations
- Johns Hopkins University Applied Physics Laboratory