Difluoramine Chemistry

Abstract

Pure 1:1 tetrafluorohydrazine was reacted with 1-hexene, cyclohexene, and 2,5-dimethyl-2,4hexadiene to give trans 1,2-bis(difluoramino) cyclohexane; cis 1,2-bis(difluoramino)cyclohexane; trans 2,5-bis(difluoramino)-2,5-dimethyl- 3-hexene; 1,2-bis(difluoramino)-n-hexane. The reactions of these compounds with a variety of reagents are under investigation. Nucleophilic reagents such as alkoxide, t-amine, and iodide primarily cause dehydrofluorination of primary and secondary difluoramines, although other reactions are also observed. Tertiary organic difluoramines apparently are not attacked by these reagents. Evidence is presented which shows that the addition reaction of tetrafluorohydrazine to olefins is reversed in the mass spectrometer. (Author)

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1961
Accession Number
AD0325602

Entities

People

  • A. Kotloby
  • A. W. Marcellis
  • C. Vogel
  • Daniel Grafstein
  • Murray S. Cohen

Tags

DTIC Thesaurus Topics

  • Addition Reactions
  • Alkanes
  • Alkenes
  • Chemical Synthesis
  • Chemistry
  • Corporations
  • Cyclic Hydrocarbons
  • Cyclohexanes
  • Cyclohexenes
  • Hydrocarbons
  • Hydrogen
  • Infrared Spectra
  • Mass Spectra
  • Mass Spectrometers
  • Materials
  • National Security
  • Organic Chemistry

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry