RESEARCH IN FLUORO-NITRO COMPOUNDS

Abstract

1-Bromo-1,1-bis(difluoramino)butane was prepared by the reaction of 1,1-dibromo-1-nitrobutane with difluoramine in the presence of fuming H2SO4. 1- Bromo-1,1-dinitrobutane did not react under these conditions. Both 1-chloro-1- nitrosocyclohexane and 1-nitro-1-nitrosocyclohexane were converted rapidly to 1, 1-bis(difluoramino)cyclohexane, indicating that the NO group is a useful leaving group for NF2 reactions. N-Methyl-Nisopropylidene-N-fluoroammonium fluoborate was prepared from t-butyldifluoramine and BF3. N-Fluoro-N-n-propylurea, was produced in the fluorination of n-propylurea together with n-propyldifluoramine and N,N-difluoro-N'-npropylurea. Fluorination of aqueous urea led to the isolation of monofluorourea. 2-Difluoraminoethylcarbamyl fluoride was prepared by fluorination of 2-imidazolidone in aqueous solution. Pure fluoroammonium perchlorate was obtained by means of vacuum sublimataon of crude product derived from the reaction of isopropyl N-fluorocarbamate and 70% HCl04.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1964
Accession Number
AD0350003

Entities

People

  • F. J. Gerhart
  • J. M. Cavallo
  • K. Baum
  • M. P. Mascari
  • V. Grakauskas

Organizations

  • Aerojet Rocketdyne Holdings

Tags

Communities of Interest

  • Advanced Electronics
  • Counter WMD
  • Weapons Technologies

DTIC Thesaurus Topics

  • Acids
  • Alkanes
  • Alkenes
  • Anhydrides
  • Aqueous Solutions
  • Chemical Products
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Contracts
  • Fluorination
  • Infrared Spectra
  • Materials
  • Organic Chemistry
  • Perchloric Acid
  • United States

Fields of Study

  • Chemistry

Readers

  • Materials Science.
  • Organic Chemistry