MASS SPECTRAL STUDIES OF KINETICS BEHIND SHOCK WAVES. I. THERMAL DISSOCIATION OF CHLORINE,

Abstract

The coupling of a shock tube to a time-of-flight mass spectrometer for the determination of kinetic data is described whereby analysis is performed every 25 microsec. The rate of dissociation of Cl2 has been measured over the temperature range 1700-3200 K under essentially isothermal and isobaric conditions with the observed rate constants in fair agreement with those obtained by the spectroscopic technique. The observed temperature dependence is less than predicted by simple collision theory with an apparent activation energy of 41 = 5 kcal./mole. (Author)

Document Details

Document Type
Technical Report
Publication Date
Aug 01, 1963
Accession Number
AD0414941

Entities

People

  • R. W. Diesen
  • W. J. Felmlee

Tags

DTIC Thesaurus Topics

  • Agreements
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chlorine
  • Collisions
  • Couplings
  • Dissociation
  • Energy
  • Heat Of Activation
  • Kinetics
  • Mass Spectrometers
  • Shock
  • Shock Tubes
  • Shock Waves
  • Spectrometers
  • Tubes

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics