THE FIRST ORDER DENSITY MATRIX FOR A PROJECTED SINGLE DETERMINANT,
Abstract
Work is initiated on a single determinant wave funccion with different orbitals for different spins. Such a function is an eigenfunction of S sub z but not, in general, of S squared. A projection operator is applied to obtain a state of pure total spin and the first order density matrix for the projected state is obtained. The resulcs are greatly simplified by choosing the orbitals in the original function so that their spacial parts are paired. The various components of the density matrix in this basis have off diagonal elements only between paired orbitals. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- May 01, 1963
- Accession Number
- AD0422045
Entities
People
- John E. Harriman
Organizations
- Uppsala University