STRUCTURE MAKERS AND BREAKERS IN WATER: PRESSURE-INDUCED CHANGES IN THE HYDRATION ATMOSPHERES OF IONS IN SOLUTION,
Abstract
The alkali metal cations may be divided into two classes. Class I consisting of Li(+) and Na(+) have four waters symmetrically arranged in their innermost solvation sheath. The application of hydrostatic pressure reduces this number to 1. Members of this class are structure makers and have positive viscosity B-coefficients. Class II consists of K(+), Rb(+), and Cs(+), which have one water in their innermost solvation sheath, which are completely dehydrated by the application of pressure, and which, due to their assymetry, are structure breakers with negative B-coefficients. Br(-) and Cl(-) tend to resemble Class II but F(-) and I(-) are exceptional in certain respects. I(-) appears to be unhydrated even at one atmosphere. (Author)
Document Details
- Document Type
- Technical Report
- Publication Date
- Sep 30, 1964
- Accession Number
- AD0449831
Entities
People
- R. A. Hörne
Organizations
- Arthur D. Little