FLUORINE NMR SPECTRA AND CONFORMATIONAL ISOMERIZATION OF 1,1-DIFLUOROCYCLOHEXANE.

Abstract

The F-19 high resolution spectrum of 1,1-difluorocyclohexane was observed at temperatures from -93 to +40 C. The rate of conformational isomerization as determined by a complete line shape analysis method for temperatures from -71 to +6 C. The activation parameters were determined for 1:1 v/v solutions in CS2 and CFCl3 at the coalescence temperature of 228 K. In the low temperature spectra of the CS2 solution, the resonance of the equutoial fluorine is shifted 15.64 ppm downfield from the axial. At temperatures above -10 C, neglect of the H-F coupling in the line shape analysis produces systematic errors in the apparent exchange rate. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jan 05, 1965
Accession Number
AD0457508

Entities

People

  • Adam Allerhand
  • J. Jonas

Organizations

  • University of Illinois Urbana–Champaign

Tags

DTIC Thesaurus Topics

  • Coalescence
  • Couplings
  • Fluorine
  • High Resolution
  • Isomerization
  • Low Temperature
  • Resonance
  • Spectra

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.
  • Quantum Chemistry
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.