NEW TYPE OF POLYMERIZATION INVOLVING ORGANOPHOSPHORUS COMPOUNDS AS CATALYSTS

Abstract

The polymerization of N-vinylcarbazole catalyzed by strong and weak Bronsted acids, diethylchlorophosphate and other compounds which hydrolyze to yield Bronsted acids, was studied under various reaction conditions in acetonitrile and methylene chloride as solvents. The polymerization is unaffected by oxygen and carbon dioxide. Although formulation of a rate expression remains inconclusive, it is evident that the cationic polymerization of N-vinylcarbazole has unusual features which facilitate a unique susceptibility to catalysis by low concentrations of acids, e.g. 40 parts per billion. The feasibility of selective sensitization to catalysis of interest was demonstrated.

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Document Details

Document Type
Technical Report
Publication Date
Feb 24, 1965
Accession Number
AD0470829

Entities

People

  • H. Scott
  • M. M. Labes
  • T. P. Konen

Organizations

  • Franklin Institute

Tags

Communities of Interest

  • C4I

DTIC Thesaurus Topics

  • Acids
  • Alcohols
  • Carbon Dioxide
  • Chemical Analysis
  • Chemical Synthesis
  • Chemistry
  • Chlorides
  • Organic Acids
  • Organic Chemistry
  • Perchloric Acid
  • Phosphorus Compounds

Fields of Study

  • Chemistry

Readers

  • Analytical Chemistry
  • Thin Film Deposition Science.