THE DEVELOPMENT AND EVALUATION OF A HYDROCARBON BINDER FOR HIGH ENERGY SOLID PROPELLANTS.

Abstract

A series of hydrogenated polybutadienes and polyisoprenes of varying backbones and molecular weights and with dicarboxy or dihydroxy terminal groups were prepared and characterized for use as solid propellant ingredients. Simultaneously a number of epoxide, aziridine, and isocyanate curing agents were characterized especially with respect to their tendency to undergo stoichiometric curing reactions in the presence of NH4ClO4. Combinations of these prepolymers and curing agents were used to prepare binders. The binders were characterized by uniaxial tensile behavior, stress relaxation, swelling, hardness, and by aging at 100 C in wet and dry air and in dry argon. Propellants with 88% solids loading were made and similarly characterized. The data allowed the selection of an isocyanate curing system, CTI and HDI, as superior to the others tested and the selection of a saturated polybutadiene terminated with secondary hydroxy groups. This system was used to make 64 lbs of propellant which was extensively characterized. (Author)

Document Details

Document Type
Technical Report
Publication Date
Feb 01, 1966
Accession Number
AD0479507

Entities

People

  • Anthony J. Di Milo
  • Duane E. Johnson

Organizations

  • Aerojet Rocketdyne Holdings

Tags

DTIC Thesaurus Topics

  • Curing
  • Curing Agents
  • High Energy
  • Hydrocarbons
  • Isocyanates
  • Molecular Weight
  • Polybutadiene
  • Propellants
  • Solid Propellants
  • Synthetic Rubber

Fields of Study

  • Materials science

Readers

  • Polymer Science and Engineering.
  • Polymer Science and Technology