Thermal Stability and Kinetic Studies of LMH-1

Abstract

The thermal stability of magnesium-doped aluminum hydride can be increased seven- to tenfold by controlled hydrolysis treatments; compatibility with propellant ingredients is also greatly improved. A 5-day n-butylamine (2% H2O) treatment at 80 C. is recommended for future use. Scanning electron photomicrographs reveal the surface characteristics of aluminum hydride crystals and show a thin coating, probably Al(OH)3, generated by hydrolysis treatments. Metallographic studies show that decomposition occurs throughout the crystal, particularly at discontinuities such as voids, cracks, and grain boundaries. Ion probe mass spectrometry shows a higher lithium content near the surface than in the interior of the crystals. Lithium aluminum hydride was extracted from AlH3- 1451 and is believed to be responsible for nucleation sites which result in the decomposition of AlH3. Pound quantities of stabilized AlH3 have been successfully used in high energy propellant formulations.

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Document Details

Document Type
Technical Report
Publication Date
Mar 01, 1970
Accession Number
AD0509735

Entities

People

  • Charles B. Roberts
  • Edwin J. Wilson

Tags

Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Alkynes
  • Chemistry
  • Crystals
  • Electron Microscopes
  • Heat Energy
  • Heavy Water
  • High Energy Propellants
  • Hydrogen
  • Mass Spectrometers
  • Mass Spectrometry
  • Materials
  • Measurement
  • Scanning Electron Microscopes
  • Spectra
  • Spectrometry
  • Spectroscopy
  • Thermal Stability

Fields of Study

  • Materials science

Readers

  • Powder metallurgy of Titanium alloys.
  • Quantum Chemistry
  • Rocket Propulsion.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene