STUDY OF CHEMICAL AGENT DECONTAMINATION SYSTEMS FOR MULTIPURPOSE USE

Abstract

Competitive hydrogen transfer studies were conducted for methyl benzoate, diisopropyl methyl phosphonate (DIMP), GB, GF and HD vs. carbon tetrachloride in each case employing phenylazotriphenylmethane (PAT) as a source of phenyl radicals. The cooxidation of GB with benzaldehyde, and of GF with 2, 2-azobis (isobutyronitrile) (AIBN), indene, and with cyclooctene was investigated at 25 C. The kinetics of the autoxidation of GF in the presence of Co(II) catalyst at 75 to 135 deg C were investigated. In addition, the autoxidation reaction was investigated in the absence of catalyst and in the presence of varying quantities of catalyst. The effect of 2,6-di-tert-butylphenol (DTBP) as an inhibitor was investigated. The autoxidation of HD in the absence and in the presence of Co(II) catalyst at 105 deg C was examined. The use of ferrous phthalocyanine as a heterogeneous catalyst for the autoxidation of GF at 25 deg C was examined. The results obtained are compared with those reported for the autoxidation of carboxylic esters.

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Document Details

Document Type
Technical Report
Publication Date
May 01, 1964
Accession Number
AD0600061

Entities

People

  • F. A. Serafin
  • H. E. Podall
  • J. L. Poling
  • S. Preis
  • Z. Oser

Organizations

  • Melpar

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Benzaldehydes
  • Benzoates
  • Carbon Tetrachloride
  • Catalysts
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Esters
  • Free Radicals
  • Heat Of Activation
  • Inhibitors
  • Materials
  • Organic Chemistry
  • Oxidation
  • Physical Properties
  • Polyethylene Glycols
  • Rate Of Consumption

Fields of Study

  • Chemistry

Readers

  • Analytical Chemistry
  • Organic Chemistry