FAR INFRARED TORSIONAL AND BENDING VIBRATIONS OF TOLUENE AND ITS DERIVATIVES AND THE BARRIER HEIGHT TO INTERNAL ROTATION.

Abstract

The far infrared spectra of ortho-, meta-, and para halogenated toluene; and butadiene- and glyoxal-type molecules was investigated. Torsional vibrations were assigned and barriers to internal rotation for methyl groups and C-C single bonds in conjugated systems have been calculated. Low bending frequencies in aromatic and acyclic conjugated molecules were observed and in some cases assigned to specific vibrational motion. Results are given on the shift in frequency resulting from changes from liquid to vapor phase. Band contours in the mid infrared region for aromatic compounds were studied in an attempt to distinguish molecules with free rotation of the methyl group. A performance comparison of Golay detectors to thermocouple is also reported. (Author)

Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1964
Accession Number
AD0605410

Entities

People

  • Foil A. Miller
  • Robert E. Witkowski
  • William G. Fateley

Tags

DTIC Thesaurus Topics

  • Aromatic Compounds
  • Butadienes
  • Detectors
  • Diffraction
  • Electromagnetic Spectra
  • Frequency
  • Frequency Shift
  • Infrared Spectra
  • Molecules
  • Phase
  • Rotation
  • Spectra
  • Thermocouples
  • Vapor Phases
  • Vibration
  • Wave Phenomena

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Spectroscopy.
  • Structural Dynamics.